8–12 Sept 2025
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New insights into isotopic activity ratios of discharges from nuclear facilities

O2.3-219
Not scheduled
15m
Forum

Forum

Oral T2.3 Atmospheric and Subsurface Radionuclide Background and Dispersion O2.3 Atmospheric and Subsurface Radionuclide Background and Dispersion

Speaker

Mr Judah Friese (Pacific Northwest National Laboratory (PNNL))

Description

Contrary to expectations based on simulations of neutron irradiation, the discharges from medical isotope production facilities (MIPFs) differ from the radioxenon isotopic activity ratios typically associated with decay chain ingrowth following a nuclear explosion whenever 131mXe is present. This discrepancy is explained in this presentation through fundamental physical principles and demonstrated using measurement data collected as part of the Source Term Analysis of Xenon (STAX) project. Another important finding from the analysis of STAX data is the correlation between specific isotopes, with the correlation coefficient varying based on the source. In cases where only one radioxenon isotope is observed, these linear dependencies can be used to estimate the expected source strength of the other isotope with the presumption that a particular model type could be the source of an event. Further relevant conclusions can be drawn from analyzing STAX data on event screening. The upper ranges of isotopic activity ratios of MIPFs and nuclear power plants are compared to the thresholds applied by the International Data Centre (IDC), which uses isotopic activity ratio screening flags to indicate a possible prompt release from a nuclear explosion.

E-mail [email protected]

Authors

Mr Judah Friese (Pacific Northwest National Laboratory (PNNL)) Mr Martin B. Kalinowski (Former CTBTO Preparatory Commission)

Co-authors

Mr Brian Schrom (Pacific Northwest National Laboratory (PNNL)) Ms Carolyn Seifert (Pacific Northwest National Laboratory (PNNL)) Charles Doll (Pacific Northwest National Laboratory (PNNL)) Mr James Ely (Pacific Northwest National Laboratory (PNNL)) Lori Metz (Pacific Northwest National Laboratory (PNNL)) Mr Matthias Auer (Instrumental Software Technologies, Inc. (ISTI)) Mihaela Rizescu (Instrumental Software Technologies, Inc. (ISTI)) Mr Paul Eslinger (Pacific Northwest National Laboratory (PNNL)) Mr Ramesh Sarathi (Pacific Northwest National Laboratory (PNNL)) Sidney Hellman (Instrumental Software Technologies, Inc. (ISTI)) Mr Theodore Bowyer (Pacific Northwest National Laboratory (PNNL))

Presentation materials

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